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广东省入库河口N2O分布和通量的时空变化
张晓萌1, 杨扬1,3*, 蔡楠2, 刘旺2, 乔永民1,3
1. 暨南大学水生生物研究所, 广州 510632; 2. 环境保护部华南环境科学研究所, 广州 510655; 3. 热带亚热带水生态工程教育部工程研究中心, 广州 510632
Spatiotemporal variations of nitrous oxide distribution and flux in estuaries of Guangdong Province
ZHANG Xiao-meng1, YANG Yang1,3, CAI Nan2, LIU Wang2, Qiao Yong-min1,3
1. Research Center of Hydrobiology, Jinan University, Guangzhou 510632, China; 2. South China Institute of Environmental sciences of the Ministry of Environmental Protection, Guangzhou 510655, China; 3. Ministry of Education Engineering Research Center of Tropical and Subtropical Aquatic Ecological Engineering, Guangzhou 510632, China
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摘要 

本研究于2011年7月(丰水期)和12月(枯水期)分别对广东省13个水库的入库河口进行调查,使用吹扫捕集-气相色谱法测定了水中N2O的浓度并用Liss&Merlivat公式估算出入库河口向大气释放N2O的水-气交换通量。结果表明,河口丰水期N2O溶存浓度范围为15.37~175.22nmol/L,平均值为(73.77±43.58)nmol/L;N2O水-气交换通量范围为0.26~5.40μmol/(m2.d),平均值是(2.53±1.94)μmol/(m2·d)。河口枯水期N2O溶存浓度范围为44.26~366.11nmol/L,平均值是(126.61±102.74)nmol/L;N2O水-气交换通量范围是0.86~21.88μmol/(m2·d),平均值是(7.50±6.65)μmol/(m2·d)。河口丰水期N2O溶存浓度和水-气交换通量明显低于枯水期。与其他研究相比,本研究区N2O溶存浓度和水-气交换通量偏低。

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张晓萌
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关键词 河口N2O分布通量时空变化    
Abstract

The concentrations and water-atmosphere fluxes of dissolved N2O were investigated in estuaries of 13 rivers of Guangdong Province during July(flooded season) and December(dry season),2011.N2O concentrations in the surface water were measured by purge and trap-gas chromatography,N2O water-atmosphere fluxes were estimated by Liss & Merlivat formula.The results demonstrated that dissolved N2O concentrations in the flooded season were 15.37-175.22 nmol/L,with an average of(73.77±43.58) nmol/L,N2O water-atmosphere fluxes in flooded season were 0.26-5.40 μmol/(m2·d),with an average of(2.53±1.94) μmol/(m2·d).While in dry season,N2O concentrations ranged from 44.26 nmol/L to 366.11 nmol/L,with an average of(126.61±102.74) nmol/L,N2O water-atmosphere fluxes ranged from 0.86 μmol/(m2·d) to 21.88 μmol/(m2·d),with an average of(7.50±6.65) μmol/(m2·).N2O concentrations and water-atmosphere fluxes of flooded season were lower than those of dry season.Compared with other studies,the estuaries in this study had lower N2O concentrations and water-atmosphere fluxes.

Key wordsestuaries    nitrous oxide    distribution    flux    spatiotemporal variation
收稿日期: 2012-06-25     
:  X142  
基金资助:国家重大科技专项(2009ZX07211-009,2008ZX07211-003)
引用本文:   
张晓萌1, 杨扬1,3*, 蔡楠2, 刘旺2, 乔永民1,3. 广东省入库河口N2O分布和通量的时空变化[J]. , 2012, 31(3): 306-311.
ZHANG Xiao-meng1, YANG Yang1,3, CAI Nan2, LIU Wang2, Qiao Yong-min1,3. Spatiotemporal variations of nitrous oxide distribution and flux in estuaries of Guangdong Province. , 2012, 31(3): 306-311.
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 http://www.ecolsci.com/CN/Y2012/V31/I3/306
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